Low Temperature Physics: 29, 185 (2003); https://doi.org/10.1063/1.1542439 (11 pages)
Физика Низких Температур: Том 29, Выпуск 3 (Март 2003), c. 250-262    ( к оглавлению , назад )

Excess electron transport in cryoobjects

D.G. Eshchenko

Institute for Nuclear Research, Moscow 117312, Russia
E-mail: eshchenko@al20.inr.troitsk.ru

V.G. Storchak

Russian Research Centre "Kurchatov Institute" 46 Kurchatov Sq., Moscow 123182, Russia

J.H. Brewer

Canadian Institute for Advanced Research and Department of Physics University of British Columbia, Vancouver, B.C., Canada V6T 2A

S.P. Cottrell and S.F.J. Cox

ISIS Facility, Rutherford Appleton Laboratory, Oxfordshire OX11 OQX, UK

Received February 19, 2002

Аннотация

Experimental results on excess electron transport in solid and liquid phases of Ne, Ar, and solid N2-Ar mixture are presented and compared with those for He. Muon spin relaxation technique in frequently switching electric fields was used to study the phenomenon of delayed muonium formation: excess electrons liberated in the m+ ionization track converge upon the positive muons and form Mu (m+e-) atoms. This process is shown to be crucially dependent upon the electron`s interaction with its environment (i.e., whether it occupies the conduction band or becomes localized in a bubble of tens of angstroms in radius) and upon its mobility in these states. The characteristic lengths involved are 10-6-10-4 cm, the characteristic times range from nanoseconds to tens microseconds. Such a microscopic length scale sometimes enables the electron spend its entire free lifetime in a state which may not be detected by conventional macroscopic techniques. The electron transport processes are compared in: liquid and solid helium (where electron is localized in buble); liquid and solid neon (where electrons are delocalized in solid and the coexistence of localized and delocalized electrons states was found in liquid recently); liquid and solid argon (where electrons are delocalized in both phases); orientational glass systems (solid N2-Ar mixtures), where our results suggest that electrons are localized in orientational glass. This scaling from light to heavy rare gases enables us to reveal new features of excess electron localization on microscopic scale. Analysis of the experimental data makes it possible to formulate the following tendency of the muon end-of-track structure in condensed rare gases. The muon-self track interaction changes from the isolated pair (muon plus the nearest track electron) in helium to multi-pair (muon in the vicinity of tens track electrons and positive ions) in argon.

PACS:
72.15.Rn - Localization effects (Anderson or weak localization)
67.40.Jg - Ions in liquid 4He
72.20.Jv - Charge carriers: generation, recombination, lifetime, and trapping
73.20.Jc - Delocalization processes